The presented study not only advances an in-depth understanding of TEMPO-based RFB applications, but also highlights the challenge of crossover of redox-active TEMPO derivative molecules applied in aqueous RFBs. . State Key Laboratory (SKL) of Biobased Transportation Fuel Technology, Department of Polymer Science & Engineering, Zhejiang University, Hangzhou 310058, China Department of Chemistry, Zhejiang University, Hangzhou 310058, China Author to whom correspondence should be addressed. The polymer P-T-S. . Water-soluble 2,2,6,6-tetramethylpiperidine-1-oxyl (TEMPO) derivatives have been frequently utilized as catholytes for aqueous redox flow batteries to achieve cost-effective renewable energy storage. However, fundamental knowledge of TEMPO derivatives is still largely underdeveloped.
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